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Molecular dynamics 3 Relaxation 2 Supercooled liquid 2 Debye law 1 Glass transition 1 Glass-former 1 Kohlrausch relaxation 1 Lennard-Jones 1 Lennard-Jones glass 1 Lennard–Jones glass 1 Mobility 1 Propensity 1 Relaxation dynamics 1 Rugged systems 1 Supercooled liquids 1
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Appignanesi, G.A. 5 Frechero, M.A. 4 Alarcón, L.M. 2 Montani, R.A. 2 Fernández, Ariel 1 Malaspina, D. 1 Montani, Rubén 1 Rodriguez Fris, J.A. 1 Schulz, E.P. 1
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Physica A: Statistical Mechanics and its Applications 5
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Spatial arrangements of particles with different mobility tendencies in a model glass-former
Malaspina, D.; Schulz, E.P.; Frechero, M.A.; … - In: Physica A: Statistical Mechanics and its Applications 388 (2009) 17, pp. 3325-3333
The use of the isoconfigurational method has enabled one to determine the existence of particles with high and low dynamic propensity (tendency to be mobile) and particles with preferred directionality for motion (directional particles) in supercooled liquids. On the other hand, dynamical...
Persistent link: https://www.econbiz.de/10010589398
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Particle mobility and metabasin exploration in model glass-formers
Appignanesi, G.A.; Frechero, M.A.; Alarcón, L.M. - In: Physica A: Statistical Mechanics and its Applications 374 (2007) 1, pp. 229-238
In this work, we assess the relevance of different range particle displacements and string motions to the metabasin (MB) dynamics of a simple glass former. We find that MB transitions are triggered by the occurrence of massive rearrangements termed as “democratic clusters” or d-clusters...
Persistent link: https://www.econbiz.de/10011062157
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Ballistic displacements within string-like motions in a supercooled liquid
Appignanesi, G.A.; Frechero, M.A.; Alarcón, L.M.; … - In: Physica A: Statistical Mechanics and its Applications 339 (2004) 3, pp. 469-481
We perform a series of molecular dynamics simulations in a binary Lennard-Jones system at temperatures close to its mode-coupling temperature, Tc. We demonstrate that the string-like movements carried out by a fraction of the particles are of ballistic nature. Depending on temperature these...
Persistent link: https://www.econbiz.de/10011058716
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Time evolution of clusters of mobile particles in a model glass former
Appignanesi, G.A.; Frechero, M.A.; Montani, R.A. - In: Physica A: Statistical Mechanics and its Applications 329 (2003) 1, pp. 41-52
In this work we investigate by means of molecular dynamics simulations the detailed time evolution of string-like cooperative motions in a binary Lennard–Jones system at temperatures close to its mode-coupling temperature, Tc. The strings will be fully geometrically and dynamically...
Persistent link: https://www.econbiz.de/10011057618
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A variational approach to relaxation in rugged free energy landscapes
Appignanesi, G.A.; Montani, Rubén; Fernández, Ariel - In: Physica A: Statistical Mechanics and its Applications 262 (1999) 3, pp. 349-358
We develop a variational principle governing the relaxation behavior of hierarchical systems. Limiting ourselves to a particular class of models amenable of a variational treatment, we study the relaxation of rugged systems whose conformation space topology deviates from ultrametricity under...
Persistent link: https://www.econbiz.de/10011058116
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